I think you would have noticed so many missing bees if they had swarmed. Opening the brood nest by adding frames was the right thing to do. But it may be too late to stop a swarm.
You might consider doing a false swarm to the Langs. Take half the brood and half the stores and move them to your Lang, leaving the other half in the TBH. If you can't determine where the queen is, make sure you get some of the capped queen cells in each after-split hive. If you can find the queen, move her to the Lang. Most of the foragers will return to the TBH.
You may be fine if you just move all the bees from TBH to Lang. Bees are constantly building queen cells and tearing them out again. But I would leave the queen cells intact, just in case you did lose your queen in a swarm.